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Contribution of nitrogen sources to streams in mixed-use watershed varies seasonally in a temperate region
Lin, Zuhong1; Liu, Junchi2; Xiao, Yong1; Yu, Chaojie1; Zhang, Jinlan1; Zhang, Tingting1
2021-11-04
发表期刊ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
ISSN0944-1344
页码13
通讯作者Xiao, Yong(xiaoyong@mail.buct.edu.cn) ; Zhang, Tingting(zhangtt@mail.buct.edu.cn)
摘要The Beiyun river flows through a hot spot region of Beijing-Tianjin-Hebei in China that serves a majority of occupants. However, the region experiences severe nitrate pollution, posing a threat to human health due to inadequate self-purification capacity. In that context, there is an urgent need to assess nitrate levels in this region. Herein, we used delta N-15-NO3, delta O-18-NO3 isotopes analysis, and stable isotope analysis model to evaluate the nitrate source apportionment in the Beiyun river. A meta-analysis was then used to compare the potential similarity of nitrate sources among the Beiyun riverine watershed and other watersheds. Results of nitrate source apportionment revealed that nitrate originated from the manure and sewage (contribution rate: 89.6%), soil nitrogen (5.9%), and nitrogen fertilizer (3.9%) in the wet season. While in the dry season, nitrate mainly originated from manure and sewage (91.6%). Furthermore, different land-use types exhibited distinct nitrate compositions. Nitrate in urban and suburban areas mostly was traced from manure and sewage (90.5% and 78.8%, respectively). Notably, the different nitrate contribution in the rural-urban fringe and plant-covered areas were manure and sewage (44.3% and 32.8%), soil nitrogen (26.9% and 35.7%), nitrogen fertilizer (23.5% and 29.4%), and atmospheric deposition (5.3% and 2.0%). Through a meta-analysis, we found nitrogen fertilizer, soil nitrogen, and manure and sewage as the main nitrate sources in the Beiyun riverine watershed or the other similar complexed watersheds in the temperate regions. Thus, this study provides a scientific basis for nitrate source apportionment and nitrate pollution preventive management in watersheds with complexed land-use types in temperate regions.
关键词Nitrate isotope Land-use Source apportionment SIAR Beijing-Tianjin-Hebei region
DOI10.1007/s11356-021-16930-8
关键词[WOS]ISOTOPE MIXING MODEL ; NITRATE SOURCES ; SOURCE APPORTIONMENT ; URBAN RIVER ; FRESH-WATER ; CHINA ; BASIN ; IDENTIFICATION ; DELTA-N-15 ; TRANSPORT
收录类别SCI
语种英语
资助项目Major Science and Technology Program for Water Pollution Control and Treatment[2018ZX07111003] ; National Natural Science Foundation of China[41977142]
项目资助者Major Science and Technology Program for Water Pollution Control and Treatment ; National Natural Science Foundation of China
WOS研究方向Environmental Sciences & Ecology
WOS类目Environmental Sciences
WOS记录号WOS:000714527500004
出版者SPRINGER HEIDELBERG
引用统计
文献类型期刊论文
条目标识符http://119.78.100.205/handle/311034/19065
专题中科院古脊椎所(2000年以后)
通讯作者Xiao, Yong; Zhang, Tingting
作者单位1.Beijing Univ Chem Technol, Res Ctr Resource & Environm, Dept Environm Sci & Engn, Beijing 100029, Peoples R China
2.Chinese Acad Sci, Inst Vertebrate Paleontol & Paleoanthropol, Key Lab Vertebrate Evolut & Human Origins, Beijing 100044, Peoples R China
推荐引用方式
GB/T 7714
Lin, Zuhong,Liu, Junchi,Xiao, Yong,et al. Contribution of nitrogen sources to streams in mixed-use watershed varies seasonally in a temperate region[J]. ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,2021:13.
APA Lin, Zuhong,Liu, Junchi,Xiao, Yong,Yu, Chaojie,Zhang, Jinlan,&Zhang, Tingting.(2021).Contribution of nitrogen sources to streams in mixed-use watershed varies seasonally in a temperate region.ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,13.
MLA Lin, Zuhong,et al."Contribution of nitrogen sources to streams in mixed-use watershed varies seasonally in a temperate region".ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH (2021):13.
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